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`(57) Abstract: Provided is a solid electrolyte
`whichis reduced in the grain boundaryresistiv-
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`electrolyte which hasa first region that is com-
`posed of a cubic garnet crystalline substance
`and a second region that is positioned around
`the first region and is composed of an amorph-
`ous substance, and wherein: the first region and
`the second region are respectively formed from
`composite oxides represented by formula (1)
`and formula (2); and the abundance ratio of
`metal atoms having an ionic radius of 78 pm or
`more gradually increases from the first region
`toward the second region. Li7\.La3..Z12A.O12 (1)
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`least one element selected from
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`WO 2017/154766
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`WO 2017/154766
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`

`WO 2017/154766
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`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
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`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
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`9
`
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`

`

`WO 2017/154766
`
`10
`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
`11
`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
`12
`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
`13
`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
`14
`
`PCT/JP2017/008463
`
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`
`

`

`WO 2017/154766
`
`15
`
`PCT/JP2017/008463
`
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`

`

`WO 2017/154766
`
`16
`
`PCT/JP2017/008463
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`

`

`WO 2017/154766
`
`17
`
`PCT/JP2017/008463
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`

`WO 2017/154766
`
`18
`
`PCT/JP2017/008463
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`

`WO 2017/154766
`
`19
`
`PCT/JP2017/008463
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`

`O 2017/154766
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`100
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`WO 2017/154766
`
`PCT/JP2017/008463
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`2/3
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`
`

`

`WO 2017/154766
`
`PCT/JP2017/008463
`
`3/3
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`[B43]
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`43
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`

`

`INTERNATIONAL SEARCH REPORT
`
`International application No.
`
`A. CLASSIFICATION OF SUBJECT MATTER
`HO1B1/06(2006.01)i, CO4B35/50(2006.01)i,
`(2010.01)i, HOIM10/0562(2010.01)i
`
`PCT/JP2017/008463
`
`HO1B1/08(2006.01)i,
`
`HO1M10/052
`
`According to International Patent Classification (IPC) or to both national classification and IPC
`B.
`FIELDS SEARCHED
`
`Minimumdocumentation searched (classification system followed by classification symbols)
`HOLB1/06-1/08, C0O4B35/50, HOIM10/052, HOI1M10/0562
`
`
`
`
`
`|C.DOCUMENTSCONSIDEREDTOBERELEVANTeeeDOCUMENTS CONSIDERED TO BE RELEVANT
`
`Relevant to claim No.
`Category*
`Citation of document, with indication, where appropriate, of the relevant passages
`JP 2013-032259 A
`(Toyota Central Research and
`
`Development Laboratories,
`Inc.
`
`da
`(14.02.2013),
`14 February 2013
`claims; examples
`(Family: none)
`
`
`
`JP 2017
`
`L3-149493 A
`
`(Honda Motor Co.
`(01.08.2013),
`O1 August 2013
`claims; examples
`(Family: none)
`
`
`
`Ltd.),
`
`
`
`Documentation searched other than minimum documentation to the extent that such documents are included in the fields searched
`
`996-2017
`
`Jitsuyo Shinan Koho
`1922-1996
`Jitsuyo Shinan Toroku Koho
`1994-2017
`Kokai Jitsuyo Shinan Koho
`1971-2017
`Toroku Jitsuyo Shinan Koho
`
`Electronic data base consulted during the international search (name of data base and, where practicable, search terms used)
`
`
` STRY (STN)
`CAplus/REG
`
`Authorized officer
`
`JP 2013-256435 A
`(Toyota Central Research and
`
`Development Laboratories,
`Inc.
`
`de
`26 December 2013
`(26.12.2013),
`
`
`
`
`
`claims; example 8
`(Family: none)
`
`
`[x] Further documents are listed in the continuation of Box C.L| See patent family annex.
`Special categories of cited documents:
`later document published after the international filing date or priority
`date and not in conflict with the application but cited to understand
`document defining the general state of the art whichis not considered
`the principle or theory underlying the invention
`be of particular relevance
`earlier application or patent but published on orafter the internationalfiling
`documentof particular relevance; the claimed invention cannot be
`considered novel or cannot be considered to involve an inventive
`date
`step when the documentis taken alonc
`document which may throw doubts on priority claim(s) or which is
`cited to establish the publication date of anothercitation or other
`documentofparticular relevance; the claimed invention cannot be
`special reason (as specified)
`considered to involve an inventive step when the documentis
`combined with one or more other such documents, such combination
`documentreferring to an oral disclosure, use, exhibition or other means
`being obvious to a person skilled in the art
`document published prior to the international filing date but later than the
`document memberof the same patent family
`priority date claimed
`
`“X”
`
`to
`
`Date of the actual completion of the international search
`Ol May 2017 (01.05.17)
`
`Date of mailing of the international search report
`16 May 2017 (16.05.17)
`
`
`Name and mailing address of the ISA/
`
`
`
`Japan Patent Office
`3-4-3,Kasumigaseki, Chiyoda-ku,
`Tokyo 100-8915, Japan
`
`Form PCT/ISA/210 (second sheet) (January 2015)
`
`

`

`INTERNATIONAL SEARCH REPORT
`
`International application No.
`
`Category*
`
`Citation of document, with indication, where appropriate, of the relevant passages
`
`Relevant to claim No.
`
`Xia TONG et al., Highly Conductive Li Garnets
`by a Multielement Doping Strategy,
`Inorganic
`Chemistry, 2015, Vol.54, No.7, pp.3600-3607
`
`
`
`
`
`
`
`
`
`EXPERIMETAL SECTION, RESULTS AND DISCUSSION
`
`
`
`ConanDOCDNTSCONSREDOBER
`
`
`
`Cc|C(Contimiation),DOCUMENTSCONSIDEREDTOBERELEVANTontinuation). DOCUMENTS CONSIDERED TO BE RELEVANT
`
`
`
`
`
`
`Toyota Central Research and
`JP 2013-037992 A
`
`Development Laboratories, Inc.),
`
`21 February 2013 (21.02.2013),
`claims; examples
`
`(Family: none)
`
`
`
`(Toyota Central Research and
`JP 2015-041573 A
`
`
`Development Laboratories, Inc.),
`02 March 2015 (02.03.2015),
`claims; examples
`& US 2015/0056519 Al
`laims; examples
`
`
`
`
`
`Form PCT/ISA/210 (continuation of second sheet) (January 2015)
`
`

`

`
`
`
`
`
`
`
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`REXLPCT /ISA4210 (2-Y) (2015185)
`
`

`

`JP 2013-256435 A (PREAH RPA)
`2013. 12. 26
`HFFAO ei PA, SehiE Bi) 8
`(Fr U—7EL)
`
`JP 2013-037992 A (PRES HEERSC)
`2013. 02. 21
`Pricbas ae 2 ee], Sebi fi)
`(Fr tT U—7EL)
`
`JP 2015-041573 A (RECAEE PA)
`2015. 03. 02
`Riri eR @ ea Be, Femi Bi
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`ROBE
`
`Xia TONG et al., Highly Conductive Li Garnets by a Multielement
`Doping Strategy,
`Inorganic Chemistry, 2015, Vol. 54, No. 7,
`pp. 3600-3607
`EXPERIMETAL SECTION, RESULTS AND DISCUSSION
`
`& US 2015/0056519 Al, Claims, Examples
`
`
`RRELPCT/ISA/210 GR2N—-YoORS)
`
`
`(201515)
`
`